Publications

Resonance energy transfer in orthogonally arranged chromophores: a question of molecular representation

Author(s)
Richard Jacobi, Leticia González
Abstract

Energy transfer between orthogonally arranged chromophores is typically considered impossible according to conventional Förster resonance energy transfer theory. Nevertheless, the disruption of orthogonality by nuclear vibrations can enable energy transfer, what has prompted the necessity for formal expansions of the standard theory. Here, we propose that there is no need to extend conventional Förster theory in such cases. Instead, a more accurate representation of the chromophores is required. Through calculations of the energy transfer rate using structures from a thermal ensemble, rather than relying on equilibrium geometries, we show that the standard Förster resonance energy transfer theory is still capable of describing energy transfer in orthogonally arranged systems. Our calculations explain how thermal vibrations influence the electronic properties of the states involved in energy transfer, affecting the alignment of transition dipole moments and the intensity of transitions.

Organisation(s)
Department of Theoretical Chemistry, Research Platform Accelerating Photoreaction Discovery
External organisation(s)
Vienna Doctoral School in Chemistry (DoSChem)
Journal
Physical Chemistry Chemical Physics
Volume
26
Pages
12299-12305
No. of pages
7
ISSN
1463-9076
DOI
https://doi.org/10.1039/d4cp00420e
Publication date
2024
Peer reviewed
Yes
Austrian Fields of Science 2012
104016 Photochemistry, 104017 Physical chemistry
ASJC Scopus subject areas
Physics and Astronomy(all), Physical and Theoretical Chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/resonance-energy-transfer-in-orthogonally-arranged-chromophores-a-question-of-molecular-representation(b026ab65-88c4-47d0-b170-c3ea46ecff43).html